@article{61,
  author = {Benji Wales and Éric Bisson and Reza Karimi and Samuel Beaulieu and Ali Ramadhan and Mathieu Giguere and ZiJian Long and Wing-Ki Liu and Jean-Claude Kieffer and François Légaré and Joseph Sanderson},
  title = {Coulomb imaging of the concerted and stepwise break up processes of OCS ions in intense femtosecond laser radiation},
  abstract = {<p>We study the break up of OCS in intense femtosecond laser radiation using the FEMPULS technique to vary the laser pulse duration from 7&nbsp;fs to 200&nbsp;fs. Newton and Dalitz plots show the progression of molecular deformation and break up for OCS<sup>3+</sup>&nbsp;and OCS<sup>4+</sup>. For increasing pulse length, the concerted three body dissociation exhibits increasing bending, and the amount of stepwise dissociation decreases. For the longest pulses however the stepwise process increases again. Both phenomena can be interpreted in terms of the effect of the laser field on lower charge states and the behaviour of a wave packet on a saddle point potential. The experiment illustrates the ability of the Coulomb imaging method to track molecular geometry and dynamics and indicates a new path to laser control of molecular parameters.</p>
},
  year = {2014},
  journal = {Journal of Electron Spectroscopy and Related Phenomena},
  volume = {195},
  chapter = {332-336},
  url = {https://www.sciencedirect.com/science/article/pii/S0368204814001121},
  doi = {10.1016/j.elspec.2014.05.003},
}