@article{72, author = {WA Bryan and Joseph Sanderson and A El-Zein and WR Newell and PF Taday and AJ Langley}, title = {Laser-induced Coulomb explosion, geometry modification and reorientation of carbon dioxide}, abstract = {

The Coulomb explosion of carbon dioxide in a 55 fs laser pulse of intensity 1.5-3 × 1016W cm-2has been studied using a variety of techniques based on time-of-flight mass spectroscopy. Covariance mapping has been used to identify Coulomb explosion channels and to measure the associated kinetic energy release. By comparing time-of-flight spectra taken with linearly and circularly polarized light, a clear signature of laser-induced reorientation is found, which is strongest for the lowest Coulombic channel. Ion-momentum imaging coupled with Monte Carlo simulation shows that the zero-point bend-angle distribution is better preserved than for longer laser pulses. However, some residue of the sequential processes dominant in much longer pulses is found.

}, year = {2000}, journal = {Journal of Physics B: Atomic, Molecular and Optical Physics}, volume = {33}, chapter = {745}, month = {2000/2/28}, url = {https://iopscience.iop.org/article/10.1088/0953-4075/33/4/312/meta}, doi = {10.1088/0953-4075/33/4/312}, }