@article{8,
  keywords = {Ultrafast Single Molecule Imaging via Femtosecond Laser},
  author = {Joseph Sanderson and Aydin Ashrafi-Belgabad and Reza Karimi and Mohammad Monfared and Kaili Tian and Parviz Parvin and Benjamin Wales and Éric Bisson and Samuel Beaulieu and Mathieu Giguere and Jean-Claude Kieffer and Philippe Lassonde and François Légaré and Heide Ibrahim},
  title = {A new path towards reconstructing real-space geometries of polyatomic molecules undergoing strong field laser-induced Coulomb explosion},
  abstract = {<p>The connection between the initial structure and final momenta of ionic fragments from the Coulomb explosion of a multiatomic molecule is investigated experimentally and theoretically for OCS. We show for the first time that an approach using time-dependent density functional theory (TDDFT) is able to rigorously model the ionization dynamics of a small molecule in the tunneling regime, reproducing the energy release and the Newton plot momentum patterns of an experiment in which OCS is ionized to the 6+ charge state using 7 fs laser pulses of 800 nm. The result suggests a pathway to unprecedented understanding of the behavior of molecules, during strong field multiple ionization and the possibility of precision imaging of real-space molecular geometries, using tabletop lasers.</p>
},
  year = {2024},
  journal = {Research Square},
  month = {2024/5/31},
  url = {https://www.researchsquare.com/article/rs-4410250/v1},
  doi = {10.21203/rs.3.rs-4410250/v1},
}