Neutron Scattering Investigations of Three-Dimensional Topological States
Physics, 200 University Ave West, Room PHY 352
Waterloo, ON, CA N2L 3G1
Magnetic skyrmions represent a unique class of topological magnet characterized by nanometric swirling spin-textures which possess a non-trivial Berry curvature. The combination of their topological stability, unique transport properties, and emergent dynamics has made skyrmions the forerunner for novel spintronic high-density memory and ultra-low power logic device applications. In this thesis, we explore the development and application of various neutron scattering tomography and structured neutron beam techniques for three-dimensional investigations of bulk magnetic topological materials and their defect-mediated dynamical phenomena. Characterization of the disordered multi-phase bulk skyrmion material, Co8Zn8Mn4, was performed through detailed SANS measurements over the entire temperature-magnetic field phase diagram of the material as a function of a dynamic skyrmion ordering sequence. 2D SANS images in combination with micromagnetic simulations reveal a novel disordered-to-ordered skyrmion square lattice transition pathway which represents a new type of non-charge conserving topological transition. In the metastable skyrmion triangular lattice phase, dynamical field-dependent skyrmion responses showed an exotic memory phase in spite of hysteresis protocols involving field-induced saturation into the ferromagnetic phase. Three-dimensional examinations of skyrmion stabilization mechanisms and their dynamical defect pathways were explored using a novel SANS tomography technique which processes multi-projection neutron scattering images as its input. Application of the technique to the ordered thermal equilibrium skyrmion triangular lattice phase yielded the first three-dimensional visualizations of a bulk skyrmion lattice. The reconstructions unveiled a host of exotic skyrmion features, such as branching, segmented, twisting, and filament structures, mediated by three-dimensional topological transitions through two different emergent monopole (MP)-antimonopole (AMP) defect pathways. Finally, the direct identification and determination of topological features and defects in bulk micromagnetic materials, without a priori knowledge of the sample, was explored using holographic approaches for the generation of neutron helical waves. Linear neutron waves in a conventional SANS setup were input on microfabricated gratings which consist of arrays of various q-fold fork-dislocation phase-gratings with nanometric spatial dimensions. Far-field scattering images exhibited doughnut intensity profiles centered on the first diffraction orders, thereby demonstrating the tunable generation of topological neutron states for phase- and topology-matched studies of quantum materials. The amalgamation of these works demonstrates the development and application of novel tools for direct investigations of bulk topological magnetic materials, while uncovering a diverse collection of skyrmion energetics, disorder-dependent dynamics, and three-dimensional topological transition defect pathways. These methods and results open the door to a new generation of neutron scattering techniques for the probing of exotic topological interactions and the complete standalone characterization of quantum materials and their topological phenomena.